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Henry entered Trininty College, Oxford in 1797 at the age of 18 and married Elizabeth Palk of Marley, Devon in 1806, a year after his father's death. Sir Henry was sheriff of Devon in 1808. He died in 1830. He was succeeded by his son Sir Walter Palk Carew. The bottles which belonged to Henry are sealed with a dexter hand apaumee and the letters H C.
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